Villainous is a series of animated shorts co-produced between Cartoon Network and Al Animation Estudios and created by Alan Ituriel, being the first Mexican animation produced for that channel. 

The cast of the English dub is this:

Black Hat - Alan Ituriel

Dr. Flug - Todd Asayer

Dementia - Melaney Sems

5.0.5 - Mark "Markiplier" Fischbach

There's only a few shorts of the series with that dub:

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